Polylactic Acid (PLA)

1/4/2008

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“Polylactic acid or polylactide (PLA) is a biodegradable, thermoplastic, aliphatic polyester derived from renewable resources, such as corn starch (in the U.S.) or sugarcanes (rest of world). Although PLA has been known for more than a century, it has only been of commercial interest in recent years, in light of its biodegradability.”
Wikipedia:  http://en.wikipedia.org/wiki/Polylactic_acid  (1/4/2008)

 

The skeletal formula of polylactic acid
Wikipedia:  http://en.wikipedia.org/wiki/Polylactic_acid  (1/4/2008)

 

Ring-opening polymerization of lactide to polylactide
Wikipedia:  http://en.wikipedia.org/wiki/Polylactic_acid  (1/4/2008)

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Notes 

“Due to the chiral nature of lactic acid, several distinct forms of polylactide exist: poly-L-lactide (PLLA) is the product resulting from polymerization of L,L-lactide (also known as L-lactide). PLLA has a crystallinity of around 37%, a glass transition temperature between 50-80 °C and a melting temperature between 173-178 °C.”
Wikipedia:  http://en.wikipedia.org/wiki/Polylactic_acid  (1/4/2008)

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“Polylactic acid can be processed like most thermoplastics into fiber (for example using conventional melt spinning processes) and film. The melting temperature of PLLA can be increased 40-50 °C and its heat deflection temperature can be increased from approximately 60°C to up to 190 °C by physically blending the polymer with PDLA (poly-D-lactide). PDLA and PLLA form a highly regular stereocomplex with increased crystallinity. The temperature stability is maximised when a 50:50 blend is used, but even at lower concentrations of 3-10% of PDLA, there is still a substantial improvement. In the latter case, PDLA acts as a nucleating agent, thereby increasing the crystallization rate. Biodegradation of PDLA is slower than for PLA due to the higher crystallinity of PDLA. PDLA has the useful property of being optically transparent.”
Wikipedia:  http://en.wikipedia.org/wiki/Polylactic_acid  (1/4/2008)

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Review Articles

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US Patents

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Journal Articles

11/21/2008

Performance Enhancement of Poly(lactic acid) and Sugar Beet Pulp Composites by Improving Interfacial Adhesion and Penetration
(8667–8675) Industrial & Engineering Chemistry Research 47 #22 (2008)

Crystallization of PLA/Thermoplastic Starch Blends
(412-418) International Polymer Processing #5 (2008)

Crystallization behavior and mechanical properties of crosslinked plasticized poly(L-lactic acid) 
(p 1530-1539)
Journal of Applied Polymer  Science 111 #3 (2009)
Abstract

10/24/2008

Solvent- and thermal-induced crystallization of poly-L-lactic acid in supercritical CO2 medium 
(p 291-300)
Journal of Applied Polymer  Science 111 #1 (2009)
Abstract

10/10/2008

Fabrication of Poly-l-lactide Biomaterials with High Mechanical Properties Using Fiber Oriented Pressing
(847 – 858) Journal of Macromolecular Science, Part B - Physics 47  #5 (2008)

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Roger D. Corneliussen
Editor
Telephone: 610 883 0055
rcorneliussen@4spe.org

www.maropolymeronline.com

Copyright 2009 by Roger D. Corneliussen